| Hundreds of innocent people nationwide have | | | | paint and bullet lead. The results of their research |
| been convicted with the help of an FBI forensic | | | | were published in U.S. Atomic Energy Commission |
| tool that was discarded over two years ago, and | | | | Reports (Lukens et al. 1970), the Journal of |
| the FBI has yet to alert the affected defendants | | | | Radioanalytical Chemistry (Guinn 1982; Guinn et al. |
| or courts, even as the window for appealing | | | | 1987), and the Journal of Forensic Sciences |
| convictions is closing. | | | | (Lukens and Guinn 1971). |
| The Basis for Compositional Bullet Lead Analysis | | | | In one research effort, the group acquired and |
| (Comparisons) | | | | analyzed samples from bullet lead manufacturers. |
| Background | | | | The results of these analyses confirmed that a |
| When the physical markings of a fired bullet | | | | cast billet poured from a pot of molten lead is |
| recovered from a crime scene are too mutilated | | | | relatively homogeneous, but that leads poured |
| for visual comparison or the firearm used in the | | | | from separate molten batches are distinguishable. |
| crime is not recovered, the bullet can be | | | | As a result, comparative bullet lead analysis has |
| compared with other bullets associated with a | | | | been adopted by laboratories and accepted by |
| suspect by its elemental composition. | | | | courts internationally (Andrasko et al. 1993; |
| When a crime-scene bullet contains the same | | | | Blacklock and Sadler 1978; Brandone and Piancone |
| analytical elemental concentrations (i.e. match in | | | | 1984; Capannesi and Sedda 1992; Cohen et al. |
| composition) as the bullets from known | | | | 1988; Desai and Parthasarathy 1983; Dufosse and |
| cartridges, a single source of these bullets cannot | | | | Touron 1998; Gillespie and Krishnan 1969; Guy and |
| by excluded. During the manufacturing processes, | | | | Pate 1973; Kishi 1987; Krishnan 1973; Krishnan and |
| thousands of lead specimens (bullets and bullet | | | | Jervis 1984; Sankar Das et al. 1978; Screenivas et |
| cores) are produced with analytically | | | | al. 1978; Suzuki and Yoshiteru 1996). |
| indistinguishable compositions. | | | | The NAA technique used at many laboratories |
| However, those lead specimens that share the | | | | has been replaced by inductively coupled |
| same composition are generally packaged within | | | | plasmaoptical emission spectroscopy (ICP-OES), |
| the same box of cartridges, or in boxes of | | | | previously known as inductively coupled |
| cartridges of the same caliber and type at the | | | | plasmaatomic emission spectroscopy (ICP-AES) |
| same manufacturing plant, on or about the same | | | | (Peters and Koons 1988). |
| date. | | | | OES was adopted because people confused AES |
| When the differences in element concentrations | | | | with auger electron spectrometry (Boss and |
| are small but analytically significant, a comparative | | | | Fredeen 1997). Since the 1970s, ICP-OES has |
| examination can be used to differentiate among | | | | been widely accepted and is the method of |
| bullets made of different alloys or to exclude a | | | | choice for most inorganic analysis (Koons 1993; |
| single source for bullets of the same alloy. | | | | Montaser and Golightly 1987). |
| Comparative bullet lead analysis was developed in | | | | One advantage of ICP-OES is its ability to |
| the early 1960s by researchers at General | | | | determine the concentrations of as many as 70 |
| Atomic (now General Activation Analysis, Inc. | | | | elements simultaneously in some samples. |
| located in Encinitas, California) under a federal | | | | ICP-OES instrumentation is used in environmental, |
| grant to develop uses for neutron activation | | | | manufacturing, research and forensic laboratories |
| analysis (NAA). | | | | throughout the world and has been used by the |
| Researchers developed procedures for analyzing | | | | FBI Laboratory in casework for the past 12 |
| such materials as gunshot primer residues, glass, | | | | years. |